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Journal Articles

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors; Project overview and progress until JFY2022

Yamano, Hidemasa; Takai, Toshihide; Emura, Yuki; Fukuyama, Hiroyuki*; Nishi, Tsuyoshi*; Morita, Koji*; Nakamura, Kinya*; Pellegrini, M.*

Nihon Kikai Gakkai 2023-Nendo Nenji Taikai Koen Rombunshu (Internet), 5 Pages, 2023/09

A research project has been conducting thermophysical property measurement of a eutectic melt, eutectic melting reaction and relocation experiments, eutectic reaction mechanism investigation, and physical model development on the eutectic melting reaction for reactor application analysis in order to simulate the eutectic melting reaction and relocation behavior of boron carbide as a control rod material and stainless steel during a core disruptive accident in an advanced sodium-cooled fast reactor designed in Japan. This paper describes the project overview and progress until JFY2022.

Journal Articles

Raman spectroscopy of eutectic melting between boride granule and stainless steel for sodium-cooled fast reactors

Fukai, Hirofumi*; Furuya, Masahiro*; Yamano, Hidemasa

Nuclear Engineering and Technology, 55(3), p.902 - 907, 2023/03

 Times Cited Count:1 Percentile:0.01(Nuclear Science & Technology)

This paper addresses reaction products and their distribution of the eutectic melting/solidifying reaction of boron carbide (B$$_{4}$$C) and stainless-steel (SS). The influence of the existence of carbon on the B$$_{4}$$C-SS eutectic reaction was investigated by comparing the iron boride (FeB)-SS reaction by Raman spectroscopy with Multivariate Curve Resolution (MCR) analysis. The scanning electron microscopy with dispersive X-ray spectrometer was also used to investigate the elemental information of the pure metals such as Cr, Ni, and Fe. In the B$$_{4}$$C-SS samples, a new layer was formed between B$$_{4}$$C/SS interface, and the layer was confirmed that the formed layer corresponded to amorphous carbon (graphite) or FeB or Fe$$_{2}$$B. In contrast, a new layer was not clearly formed between FeB and SS interface in the FeB-SS samples.

Journal Articles

Experimental study on reaction behavior between control rod material and molten stainless steel for core disruptive accidents of sodium-cooled fast reactors

Emura, Yuki; Kamiyama, Kenji; Yamano, Hidemasa

Dai-26-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 4 Pages, 2022/07

no abstracts in English

Journal Articles

In situ EELS and TEM observation of boron carbide(B$$_{4}$$C) during hydrogen- and hilium-ion bombardments

Kushita, Kohei; Hojo, Kiichi; Furuno, Shigemi

Microsc. Microanal. Microstruct., 6, p.149 - 157, 1995/02

 Times Cited Count:13 Percentile:65.31(Microscopy)

no abstracts in English

Journal Articles

Effect of neutron irradiation on length, thermal expansivity and thermal conductivity of boronated graphites

Matsuo, Hideto; Kobayashi, Fumiaki; Sawa, Kazuhiro

Tanso, 0(159), p.185 - 191, 1993/00

no abstracts in English

Oral presentation

Fuel and NFBC assemblies design for the next generation sodium-cooled fast reactor, 2; Optimization of a radial shielding structure

Saito, Hiroyuki*; Higurashi, Koichi*; Masuyama, Daisuke*; Oki, Shigeo; Ohgama, Kazuya; Maeda, Seiichiro

no journal, , 

no abstracts in English

Oral presentation

High-temperature reaction of B$$_{4}$$C with (Pu,U)O$$_{2}$$

Otobe, Haruyoshi; Hayashi, Hirokazu; Takano, Masahide

no journal, , 

The high-temperature reaction of B$$_{4}$$C with U$$_{0.93}$$Pu$$_{0.07}$$O$$_{2}$$ has been investigated. The samples were prepared by mixing B$$_{4}$$C and U$$_{0.93}$$Pu$$_{0.07}$$O$$_{2}$$ powders for the molar ratio of 1 to 1 and 1 to 4 and pressing them into disks. The samples heated at 1333 or 1473 K in Ar gas were identified to be the fluorite-type phases like UO$$_{2}$$ by the powder X-ray diffraction method, independently of the molar ratio of B$$_{4}$$C to U$$_{0.93}$$Pu$$_{0.07}$$O$$_{2}$$ and the heating temperature. The formation of PuBO$$_{3}$$ was not discernable in the X-ray diffraction patterns. The samples heated at 1473 K in He-4%H$$_{2}$$ gas were also the fluorite-type phases, independently of the molar ratio of B$$_{4}$$C to U$$_{0.93}$$Pu$$_{0.07}$$O$$_{2}$$ (1 to 1 or 1 to 4). On the other hand, the samples heated at 1333 K in He-4%H$$_{2}$$ gas were composed of not only fluorite-type phases but also B$$_{4}$$C phases.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 6; Thermophysical properties of 10mass%B$$_{4}$$C-SS eutectic materials in the solid state

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

no journal, , 

This study describes estimation results of thermophysical properties of stainless steel containing boron carbide (B$$_{4}$$C-SS) in the solid state. Obtained results will be applied to development of physical models that explain the eutectic melting behavior.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 7; Density and surface tension of 10mass%B$$_{4}$$C-SS eutectic molten materials

Fukuyama, Hiroyuki*; Higashi, Hideo*; Yamano, Hidemasa

no journal, , 

To develop thermophysical property model to simulate eutectic reaction behavior of B$$_{4}$$C as control rod material and stainless steel: SUS316L (SS) in core disruptive accident of sodium-cooled fast reactor, thermophysical property measurement of B$$_{4}$$C-SS melt has been systematically conducted with very high temperature physical property measurement system (PROSPECT). This fiscal year's paper reports measurement results of density and surface tension of 10mass%B$$_{4}$$C-SS melt.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 9; Viscosity measurement of 10mass%B$$_{4}$$C-SS eutectic molten material

Nishi, Tsuyoshi*; Ota, Hiromichi*; Yamano, Hidemasa

no journal, , 

It is necessary to obtain viscosity data of eutectic molten material of boron carbide (B$$_{4}$$C) and stainless steel (SS) for severe accident analyses. In this study, continuing from viscosity measurement of 5mass%B$$_{4}$$C-SS eutectic melt which was reported in JFY 2017, viscosity measurement of 10mass%B$$_{4}$$C-SS eutectic melt and its data verification have been conducted. This paper reports their results.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 16; Immersion tests of B$$_{4}$$C into molten stainless steel

Emura, Yuki; Kamiyama, Kenji; Yamano, Hidemasa

no journal, , 

In core disruptive accidents of sodium-cooled fast reactors, boron carbide used as the control material may melt into molten stainless steel and be widely transferred to the inside and outside of the core region. In this study, a series of tests was conducted to acquire the data regarding melting rate of boron carbide into molten stainless steel and its results were considered.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 14; Emissivity, heat capacity and thermal conductivity of 7mass% B$$_{4}$$C-SS eutectic molten material

Higashi, Hideo*; Fukuyama, Hiroyuki*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel (SS)) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the emissivity, thermal capacity, and thermal conductivity of the molten material of 7mass% B$$_{4}$$C-SS measured with High-Temperature Thermophysical Property Measurement System (PROSPECT) employing noncontact laser modulation calorimetry.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 13; Density and surface tension of 7mass% B$$_{4}$$C-SS eutectic molten materials

Fukuyama, Hiroyuki*; Higashi, Hideo*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel: SUS316L (SS)) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the density and surface tension of the molten compound of 7mass% B$$_{4}$$C-SS systematically measured with the High-Temperature Thermophysical Property Measurement System (PROSPECT).

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 20; Thermophysical properties of 17mass%B$$_{4}$$C-SS eutectic in the solid state

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

no journal, , 

For contribute to the CDA analysis computer codes development for the SS-B$$_{4}$$C liquification and relocation behavior, this paper described the measurement results of the thermophysical properties of SS-B$$_{4}$$C in the solid phase

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 21; Density and surface tension of 2.5mass% B$$_{4}$$C-SS eutectic molten materials

Fukuyama, Hiroyuki*; Higashi, Hideo*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel: SUS316L (SS)) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the density and surface tension of the molten compound of 2.5mass% B$$_{4}$$C-SS systematically measured with the High-Temperature Thermophysical Property Measurement System (PROSPECT).

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 22; Emissivity, heat capacity and thermal conductivity of 2.5mass% B$$_{4}$$C-SS eutectic molten material

Higashi, Hideo*; Fukuyama, Hiroyuki*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel: SS) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the emissivity, thermal capacity, and thermal conductivity of the molten material of 2.5mass% B$$_{4}$$C-SS measured with High-Temperature Thermophysical Property Measurement System (PROSPECT) employing noncontact laser modulation calorimetry.

Oral presentation

Viscosity measurements of molten stainless-steel containing boron-carbide

Nishi, Tsuyoshi*; Ota, Hiromichi*; Kokubo, Hiroki*; Sato, Rika*; Yamano, Hidemasa

no journal, , 

In this study, the viscosities of the molten SS (SUS316L), 2.5mass%B$$_{4}$$C-SS, 5.0mass%B$$_{4}$$C-SS, 7.0mass%B$$_{4}$$C-SS and 10mass%B$$_{4}$$C-SS alloys were measured by the oscillating crucible method. The viscosity measurements of the molten SS, 2.5mass%B$$_{4}$$C-SS and 5mass%B$$_{4}$$C-SS, 7mass%B$$_{4}$$C-SS and 10mass%B$$_{4}$$C-SS alloys were performed in the temperature range from 1613 to 1793 K, from 1713 to 1793 K, and from 1793 to 1823 K, respectively. In these results, the viscosity increased with B$$_{4}$$C components in the B$$_{4}$$C components range from 0 to 7.0mass%. The equation of viscosity of molten B$$_{4}$$C-SS alloys was estimated by using the experimental data of the molten 2.5mass%B$$_{4}$$C-SS and 5.0mass%B$$_{4}$$C-SS, and 7.0mass%B$$_{4}$$C-SS in the temperature range from 1713 to 1793 K. The equation of viscosity of molten SS+B$$_{4}$$C alloys was determined as follows. y=Ax+B, A=0.0302, B=-9.881$$times$$10$$^{-4}$$T+2.546, where x is the B$$_{4}$$C component and T is the temperature. The uncertainty of the equation is 2.5%.

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 26; Density and surface tension of 15mass% B$$_{4}$$C-SS eutectic molten materials

Fukuyama, Hiroyuki*; Higashi, Hideo*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel: SUS316L (SS)) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the liquidus temperature, density and surface tension of the molten compound of 15mass% B$$_{4}$$C-SS systematically measured with the High-Temperature Thermophysical Property Measurement System (PROSPECT).

Oral presentation

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 27; Normal spectral Emissivity, heat capacity and thermal conductivity of 15mass% B$$_{4}$$C-SS eutectic molten material

Higashi, Hideo*; Fukuyama, Hiroyuki*; Yamano, Hidemasa

no journal, , 

The purpose of this study is to develop the thermophysical property model needed to simulate the behavior of the eutectic compound of the control rod material (boron carbide (B$$_{4}$$C)) and the structural material of a reactor vessel (stainless steel: SS) during a core disruptive accident in a sodium-cooled fast reactor. This paper describes the emissivity, thermal capacity, and thermal conductivity of the molten material of 15mass% B$$_{4}$$C-SS measured with High-Temperature Thermophysical Property Measurement System (PROSPECT) employing noncontact laser modulation calorimetry.

28 (Records 1-20 displayed on this page)